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Imine

An imine is a functional group or chemical compound containing a carbon-nitrogen double bond. An imine can be synthesised by nucleophilic addition from a ketone or aldehyde and ammonia or an amine to a hemiaminal -C(OH)(NHR)- followed by elimination of water to the imine.

Synthesis

  • The addition of ammonia to an aldehyde or ketone does not lead to a stable imine. The reaction of formaldehyde and ammonia yields hexamethylenetetramine .
  • Addition reactions with primary amines give stable imines
  • but with an aryl substituent on nitrogen, (the imine is then called a Schiff base) the imine is truly stable.
  • A secondary amine lacks hydrogen and elimination of water is not possible. The hemiaminal intermediate is not stable and
    • with no alpha hydrogen present it proceeds to form a aminal
    • with alpha hydrogen present it proceeds to form an enamine
  • note that addition of carbonyl compounds to the salt of an amine yields the corresponding Mannich base


Reactions

References

  • March Jerry; (1985). Advanced Organic Chemistry reactions, mechanisms and structure (3rd ed.). New York: John Wiley & Sons, inc. ISBN 0-471-85472-7
01-04-2007 01:16:19
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